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CTerminal angle M-N-N. dBridge angle M-N-N. •The angle Re-N-N. rThe angle Mo-N-N. 8 There are two structural units of the type in each molecule. hThe angle Co-N-N. 'The angle Mg-N-N. : (A) Girolami GS et al. (1983). (B) Poveda ML et al. (1983). (CI,C2) Carmona E et al. (1983a, 1983b). (D) Sato Metal. (1978). (El,E2) Uchida T et al. (1971, 1975). (F) Anderson SN et al. (1986). (G) Morris RH et al. (1984). (H) Yoshida T et al. (1984). (II, 12, 13, 14) Davis BR eta!. (1969a, 1969b, 1970, 1971). (J) Carvalho FN et al.
4. Charge densities on both the exo-(N-1) and endo-(N-2) nitrogen atoms in mononuclear transdouble-end-on coordination compound (N-1 - N-2-M-3 - N-2'- N-1') of a d6 configuration as a function of b. q 1 is the charge density on N-1 and q 2 is for N-2. , N-1 is always more negative than N-2), the N-2 atom is the first to be attacked by electrophilic groups, including H +. The higher activity of the exo-N atom is entirely analogous to the single end-on-coordinated N 2 complexes, in agreement with the X-ray photoelectron spectroscopic studies (Brant and Feltham 1977).
N) Fergusson JE eta! (1972). (0) Camenzind MJ et at. (1988). (P) Gallop MA eta!. (1984). (Q) Cruz-Garrity D eta!. (1988). (R) Enemark JH eta!. (1968). (S) Klein HF et at. (1978). (T) Hoffman PR eta!. (1976). (U)Thorn DL et at. (1979). (VI, V2) Sannar RD eta!. (1976a, 1976b). (W) Berry DH et al. (1988). (X) Zeinstra JD et al. (1979). (Y) Edema JJH et al. (1989). (Z) Turner HU et al. (Abl,Ab2,Ab3,Ab4)Churchill MRet a!. (1981, 1982, 1984, 1986). (Be) Schroch RR et at. (1988). (Cd) Denholm Setal. (1987).